Spatiotemporal mode-locking creates great opportunity for pulse energy scaling and nonlinear optics research in fiber. Until now, spatiotemporal mode-locking has only been realized in normal-dispersion dissipative soliton and similariton fiber lasers. In this paper, we demonstrated the first experimental realization of a spatiotemporally mode-locked soliton laser in mid-infrared fluoride fiber with anomalous dispersion. The mode-locked fluoride fiber oscillator directly generated a record pulse energy of 16.1 nJ and peak power of 74.6 kW at 2.8 μm wavelength. This work extends the spatiotemporal mode-locking to soliton fiber lasers and should have a wide interest for the laser community.

We report on a grating-free fiber chirped pulse amplifier (CPA) at 2.8 μm for the first time. The CPA system adopted Er:ZBLAN fiber with large anomalous dispersion as the stretcher and germanium (Ge) rods as the compressor with a compact structure. High-energy picosecond pulses of 2.07 μJ were generated at the repetition rate of 100 kHz. Using highly dispersive Ge rods, the amplified pulses were compressed to 408 fs with a pulse energy of 0.57 μJ, resulting in a peak power of approximately 1.4 MW. A spectral broadening phenomenon in the main amplifier was observed, which was caused by the special gain shape of the Er:ZBLAN fiber amplifier in operation and confirmed by our numerical simulation. This compact fiber CPA system at 2.8 μm will be practical and meaningful for application fields.

Dissipative solitons have been realized in mode-locked fiber lasers in the theoretical framework of the Ginzburg–Landau equation and have significantly improved the pulse energy and peak power levels of such lasers. It is interesting to explore whether dissipative solitons exist in optical parametric oscillators in the framework of three-wave coupling equations in order to substantially increase the performance of optical parametric oscillators. Here, we demonstrate a temporal-filtering dissipative soliton in a synchronously pumped optical parametric oscillator. The temporal-gain filtering of the pump pulse combined with strong cascading nonlinearity and dispersion in the optical parametric oscillator enables the generation of a broad spectrum with a nearly linear chirp; consequently, a significantly compressed pulse and high peak power can be realized after dechirping outside the cavity. Furthermore, we realized, for the first time, dissipative solitons in an optical system with a negative nonlinear phase shift and anomalous dispersion, extending the parameter region of dissipative solitons. The findings may open a new research block for dissipative solitons and provide new opportunities for mid-infrared ultrafast science.

文中首次提出并验证了基于腔内色散管理实现飞秒光参量振荡器（OPO）光谱净化和稳定性提升的方法。对于高功率飞秒OPO，输出脉冲通常具有随时间无序变化的宽带不规则光谱，输出功率波动较大。利用铌酸锂（LiNbO₃）晶体在腔内引入额外的负色散，通过泵浦脉冲的时间滤波效应实现了干净平滑的窄光谱近转换极限的飞秒脉冲输出，光谱稳定性和功率稳定性得到了极大改善。该方法是一种实现飞秒OPO光谱净化和稳定性提升的灵活简便的方法，对于发展高功率的超短脉冲OPO具有重要的应用价值。

We demonstrated a femtosecond mode-locked Er:ZrF₄-BaF₂-LaF₃-AlF₃-NaF (Er:ZBLAN) fiber laser at 2.8 μm based on the nonlinear polarization rotation technique. The laser generated an average output power of 317 mW with a repetition rate of 107 MHz and pulse duration as short as 131 fs. To the best of our knowledge, this is the shortest pulse generated directly from a mid-infrared mode-locked Er:ZBLAN fiber laser to date. Numerical simulation and experimental results confirm that reducing the gain fiber length is an effective way to shorten the mode-locked pulse duration in the Er:ZBLAN fiber laser. The work takes an important step towards sub-100-fs mid-infrared pulse generation from mode-locked Er:ZBLAN fiber lasers.

The mode-locked fluoride fiber laser (MLFFL) is an exciting platform for directly generating ultrashort pulses in the mid-infrared (mid-IR). However, owing to difficulty in managing the dispersion in fluoride fiber lasers, MLFFLs are restricted to the soliton regime, hindering pulse-energy scaling. We overcame the problem of dispersion management by utilizing the huge normal dispersion generated near the absorption edge of an infrared-bandgap semiconductor and promoted MLFFL from soliton to breathing-pulse mode-locking. In the breathing-pulse regime, the accumulated nonlinear phase shift can be significantly reduced in the cavity, and the pulse-energy-limitation effect is mitigated. The breathing-pulse MLFFL directly produced a pulse energy of 9.3 nJ and pulse duration of 215 fs, with a record peak power of 43.3 kW at 2.8 μm. Our work paves the way for the pulse-energy and peak-power scaling of mid-IR fluoride fiber lasers, enabling a wide range of applications.

In past years, rare-earth-doped fluoride fiber lasers (FFLs) have developed rapidly in the mid-infrared (mid-IR) region. However, due to the lack of fiber optic devices and challenge of fluoride fiber splicing, most mid-IR FFLs have been demonstrated with free-space optic elements, limiting the advantages of all-fiber lasers for flexible delivery, stability, and compactness. Here, we report, to the best of our knowledge, the first pulsed all-fiber FFL in the mid-IR region. By taking advantage of the integration of black phosphorus flake, stable Q-switched and mode-locked pulses were obtained at 2.8 μm wavelength. We believe that this all-fiber design will promote the application of pulsed FFL in the mid-IR region.

High-power ultrafast fiber lasers operating at the 2 μm wavelength are extremely desirable for material processing, laser surgery, and nonlinear optics. Here we fabricated large-core (LC) double-cladding Tm-doped silica fiber via the sol-gel method. The sol-gel-fabricated Tm-doped silica (SGTS) fiber had a large core diameter of 30 μm with a high refractive index homogeneity (Δn=2×10 4). With the newly developed LC SGTS fiber as the gain fiber, high-power mode-locking was realized. By using a semiconductor saturable absorber mirror (SESAM) as a mode locker, the LC SGTS fiber oscillator generated mode-locked pulses with an average output power as high as 1.0 W and a pulse duration of 23.9 ps at the wavelength of 1955.0 nm. Our research results show that the self-developed LC Tm-doped silica fiber via the sol-gel method is a promising gain fiber for generating high-power ultrafast lasers in the 2 μm spectral region.

We report a continuous-wave Er:ZBLAN fiber laser with the operation wavelength reaching 3.68 μm. The mid-infrared Er:ZBLAN fiber laser is pumped with the dual-wavelength sources consisting of a commercial laser diode at 970 nm and a homemade Tm-doped fiber laser at 1973 nm. By increasing the launched pump power at 1973 nm, the laser wavelength can be switched from 3.52 to 3.68 μm. The maximum output power of 0.85 W is obtained with a slope efficiency of 25.14% with respect to the 1973 nm pump power. In the experiment, the laser emission at 3.68 μm is obtained with a significant power of 0.62 W, which is the longest emission wavelength in free-running Er:ZBLAN fiber lasers.